Here we developed a fastgreen process of micro-plasma system for three-dimensional porous nanomaterials on low-cost paper substrates. The characteristics are low-cost, flexible,high-stability. It has three major applications, including increasing Raman measument, the detection process can be used with portable Raman spectroscopy for fast sensing,it can quickly analyze pesticides, food, drugs, etc. In addition, it can be equipped with boron nitride for high hydrogen productionhigh pollution biodegradationother applications.